One of the coolest pieces of hardware I picked up in the last while was a VIC-REL "cartridge". It isn't really a cartridge because it plugs into the user port, but it is in a VIC20-style cartridge case. In fact, it was designed for the VIC-20, and the manual is written for VIC20 users, but there is a short appendix for what POKEs to substitute if you're using it on a Commodore 64.
The VIC-REL gives you 6 relay outputs and 2 inputs. So, I used four of the relay outputs to simulate moving levers in my remote control truck transmitter.

The software is very simple. It's a short BASIC program (available here) that initializes the VIC-REL with two POKEs (one to set the User port to 6 outputs and 2 inputs) and one to turn all the outputs off.
From there, a simple menu lets you set the outputs individually, or drive the truck from Joystick Port 2 (very fun!!!) You can also write short BASIC programs to make the truck follow a predetermined timed pattern so it drives itself, which is really neat.